Dental Materials
Volume 25, Issue 1 , Pages 26-32 , January 2009

Effect of propionaldehyde or 2,3-butanedione additives on the mechanical properties of Bis-GMA analog-based composites

This paper is dedicated to the memory of Dr. Sid Kalachandra, who loved ‘polymer science’ and routinely shared his keen wit.

  • Anuradha Prakki

      Affiliations

    • Center for Oral and Systemic Diseases, University of North Carolina at Chapel Hill, Chapel Hill, NC, USA
    • Department of Restorative Dentistry, University of Toronto, Faculty of Dentistry, Toronto, Ontario, Canada
    • ,
  • Patricia Nobrega Rodrigues Pereira

      Affiliations

    • Department of Operative Dentistry, University of North Carolina at Chapel Hill, Chapel Hill, NC, USA
    • ,
  • Sid Kalachandra

      Affiliations

    • Center for Oral and Systemic Diseases, University of North Carolina at Chapel Hill, Chapel Hill, NC, USA
    • Corresponding Author InformationCorresponding author at: Biomaterials, Center for Oral and Systemic Diseases, Room 3130, Old Dental Building, School of Dentistry, CB #7455, University of North Carolina at Chapel Hill, Chapel Hill, NC 27599-7455, USA. Tel.: +1 919 966 4545; fax: +1 919 966 7537.

Received 4 February 2008 ,Revised 27 April 2008 ,Accepted 10 May 2008.

References 

  1. Bowen RL. Dental filling material comprising vinyl silane treated fused silica and a binder consisting of the reaction product of bis phenol and glycidyl acrylate. US Patent 3,066,112;1962.
  2. Moszner N, Salz U. New developments of polymeric dental composites. Prog Polym Sci. 2001;26:535–576
  3. Ferracane JL. Hygroscopic and hydrolytic effects in dental polymer networks. Dent Mater. 2006;22:211–222
  4. Davy KWM, Kalachandra S, Pandain MS, Braden M. Relationship between composite matrix molecular structure and properties. Biomaterials. 1998;19:2007–2014
  5. Kalachadra S, Turner DT. Water sorption of polymethacrylate networks: Bis-GMA/TEGDM copolymers. J Biomed Mater Res. 1987;21:329–338
  6. Pereira SG, Teresa GN, Kalachandra S. Low viscosity dimethacrylate comonomer compositions [Bis-GMA and CH3Bis-GMA] for novel dental composites; analysis of the network by stray-field MRI, solid-state NMR and DSC & FTIR. Biomaterials. 2002;23:3799–3806
  7. Pereira SG, Osorio R, Toledano M, Nunes TG. Evaluation of two Bis-GMA analogues as potential monomer diluents to improve the mechanical properties of light-cured composite resins. Dent Mater. 2005;21:823–830
  8. Pereira SG, Osorio R, Toledano M, Cabrerizo-Vilchez MA, Nunes TG, Kalachandra S. Novel light-cured resins and composites with improved physicochemical properties. Dent Mater. 2007;23:1189–1198
  9. Kalachandra S, Taylor DF, Deporter CD, Grubbs HJ, McGrath JE. Polymeric materials for composite matrices in biological environments. Polymer. 1993;34:778–782
  10. Sankarapandian M, Xu Q, McGrath JE, Taylor DF, Kalachandra S. Influence of resin molecular structure on the processibility and physical behavior of a dental composite matrix. J Adv Mater. 1996;28:59–63
  11. Prakki A, Tallury P, Mondelli RFL, Kalachandra S. Influence of additives on the properties of Bis-GMA/Bis-GMA analog comonomers and corresponding copolymers. Dent Mater. 2007;23:1199–1204
  12. Shobha HK, Sankarapandian M, Sun Y, Kalachandra S, McGrath JE, Taylor DF. Effect of dilution on the kinetics of cross-linking thermal polymerization of dental composite matrix resins. J Mater Sci Mater Med. 1997;8:583–586
  13. Peutzfeldt A. Retention of propanal and diacetyl in experimental resins. Acta Odontol Scand. 1997;55:94–100
  14. Peutzfeldt A, Asmussen E. Influence of aldehydes on selected mechanical properties of resin composites. J Dent Res. 1992;71:1522–1524
  15. Peutzfeldt A, Asmussen E. Influence of ketones on selected mechanical properties of resin composites. J Dent Res. 1992;71:1847–1850
  16. Peutzfeldt A, Asmussen E. In vitro wear, hardness, and conversion of diacetyl-containing and propanal-containing resin materials. Dent Mater. 1996;12:103–108
  17. Lovell LG, Lu H, Elliott JE, Stansbury JW, Bowman CN. The effect of cure rate on the mechanical properties of dental resins. Dent Mater. 2001;17:504–511
  18. Peutzfeldt A. Quantity of remaining double bonds of propanal-containing resins. J Dent Res. 1994;73:1657–1662
  19. Sankarapandian M, Shobha HK, Kalachandra S, McGrath JE, Taylor DF. Characterization of some aromatic dimethacrylates for dental composite applications. J Mater Sci Mater Med. 1997;8:465–468
  20. Atai M, Ahmadi M, Babanzadeh S, Watts D. Synthesis, characterization, shrinkage and curing kinetics of a new low-shrinkage urethane dimethacrylate monomer for dental applications. Dent Mater. 2007;23:1030–1041
  21. Arcis RW, Lopez-Macipe A, Toledano M, Osorio E, Rodriguez-Clemente R, Murtra J, et al. Mechanical properties of visible light cured resins reinforced with hydroxyapatite for dental restoration. Dent Mater. 2002;18:49–57
  22. Peutzfeldt A, Asmussen E. Modulus of resilience as predictor for clinical wear of restorative materials. Dent Mater. 1992;8:146–148
  23. St-Georges AJ, Swift EJ, Thompson JY, Heymann HO. Irradiance effects on the mechanical properties of universal hybrid and flowable hybrid resin composites. Dent Mater. 2003;19:406–413
  24. Peutzfeldt A, Asmussen E. Effect of propanal and diacetyl on quantity of remaining double bonds of chemically cured Bis-GMA/TEGDMA resins. Eur J Oral Sci. 1996;104:309–312
  25. Sun GJ, Chae KH. Properties of 2,3-butanedione and 1-phenyl-1,2-propanedione as new photosensitizers for visible light cured dental resin composites. Polymer. 2000;41:6205–6212
  26. Ferracane JL, Greener EH. The effect of resin formulation on the degree of conversion and mechanical properties of dental restorative resins. J Biomed Mater Res. 1986;20:121–131
  27. Stansbury JW. Curing dental resins and composites by photopolymerization. J Esthet Dent. 2000;12:300–308
  28. Darvell BW. Materials science for dentistry. Hong Kong: BW Darvell; 2002;p. 19–20
  29. Yoshida K, Greener EH. Effects of two amine reducing agents on the degree of conversion and physical properties of an unfilled light-cured resin. Dent Mater. 1993;9:246–251
  30. Nie J, Lindén LA, Rabek JF, Fouassier JP, Morlet-Savary F, Scigalski F, et al. A reappraisal of the photopolymerization kinetics of triethyleneglycol dimethacrylate initiated by camphorquinone-N,N-dimethyl-p-toluidine for dental purposes. Acta Polym. 1998;49:145–161
  31. Rueggeberg FA, Ergle JW, Lockwood PE. Effect of photoinitiator level on properties of a light-cured and post-cure heated model resin system. Dent Mater. 1997;13:360–364
  32. Knobloch LA, Kerby RE, Seghi R, Putten MV. Two body wear resistance and degree of conversion of laboratory-processed composite materials. Int J Prosthodont. 1999;12:432–438
  33. Zidan O, Asmussen E, Jorgensen KD. Tensile strength of restorative resins. Scand J Dent Res. 1980;88:285–289

PII: S0109-5641(08)00131-0

doi: 10.1016/j.dental.2008.05.002

Dental Materials
Volume 25, Issue 1 , Pages 26-32 , January 2009

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